Kalai may refer to:
People
- Adam Tauman Kalai, American computer scientist
- Ehud Kalai, prominent American game theorist and mathematical economist
- Gil Kalai (born 1955), Henry and Manya Noskwith Professor of Mathematics at the Hebrew University of Jerusalem
- Hanoch Kalai (1910–1979), member of Irgun and Lehi and an expert on the Hebrew language
- Iosif Kalai (born 1980), Romanian football player of Hungarian ethnicity
- Leslie Kalai (born 1984), Papua New Guinean footballer who is a goalkeeper
- Yael Tauman Kalai, Israeli-American cryptographer
Places
- Kalai, Iran, village in Gilan Province, Iran
- Kalai, Cambodia, commune in Ou Chum District in northeast Cambodia
- Kalai Upazila, Upazila of Joypurhat District in the Division of Rajshahi, Bangladesh
Other uses
- Kaivantha Kalai, a 2006 South Indian Tamil film written and directed by Pandiarajan
- Kalai Arasi, a 1963 Tamil-language adventure science fiction-comedy film
- Kalai (process), a metalworking process
- Koloi or Kalai, a scheduled tribe in Tripura, India
- Varma kalai, a martial art and esoteric healing art originating from ancient Tamil Nadu in South India
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